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  4. Urinary analysis of four testosterone metabolites and pregnanediol by gas chromatography-combustion-isotope ratio mass spectrometry after oral administrations of testosterone.
 
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Titre

Urinary analysis of four testosterone metabolites and pregnanediol by gas chromatography-combustion-isotope ratio mass spectrometry after oral administrations of testosterone.

Type
article
Institution
UNIL/CHUV/Unisanté + institutions partenaires
Périodique
Journal of Analytical Toxicology  
Auteur(s)
Maître, A.
Auteure/Auteur
Saudan, C.
Auteure/Auteur
Mangin, P.
Auteure/Auteur
Saugy, M.
Auteure/Auteur
Liens vers les personnes
Saugy, Martial  
Mangin, Patrice  
Saudan, Christophe  
Liens vers les unités
Médecine légale (CURML)  
Unité romande de médecine forensique (URMF)  
Laboratoire d'analyse du dopage (LAD)  
ISSN
0146-4760
Statut éditorial
Publié
Date de publication
2004
Volume
28
Numéro
6
Première page
426
Dernière page/numéro d’article
31
Peer-reviewed
Oui
Langue
anglais
Notes
Publication types: Clinical Trial ; Journal Article ; Research Support, Non-U.S. Gov't - Publication Status: ppublish
Résumé
The most frequently used method to demonstrate testosterone abuse is the determination of the testosterone and epitestosterone concentration ratio (T/E ratio) in urine. Nevertheless, it is known that factors other than testosterone administration may increase the T/E ratio. In the last years, the determination of the carbon isotope ratio has proven to be the most promising method to help discriminate between naturally elevated T/E ratios and those reflecting T use. In this paper, an excretion study following oral administration of 40 mg testosterone undecanoate initially and 13 h later is presented. Four testosterone metabolites (androsterone, etiocholanolone, 5 alpha-androstanediol, and 5 beta-androstanediol) together with an endogenous reference (5 beta-pregnanediol) were extracted from the urines and the delta(13)C/(12)C ratio of each compound was analyzed by gas chromatography-combustion-isotope ratio mass spectrometry. The results show similar maximum delta(13)C-value variations (parts per thousand difference of delta(13)C/(12)C ratio from the isotope ratio standard) for the T metabolites and concomitant changes of the T/E ratios after administration of the first and the second dose of T. Whereas the T/E ratios as well as the androsterone, etiocholanolone and 5 alpha-androstanediol delta(13)C-values returned to the baseline 15 h after the second T administration, a decrease of the 5 beta-androstanediol delta-values could be detected for over 40 h. This suggests that measurements of 5 beta-androstanediol delta-values allow the detection of a testosterone ingestion over a longer post-administration period than other T metabolites delta(13)C-values or than the usual T/E ratio approach.
Sujets

Administration, Oral

Adult

Algorithms

Androgens

Biotransformation

Carbon Dioxide

Gas Chromatography-Ma...

Humans

Male

Mass Spectrometry

Pregnanediol

Solvents

Testosterone

PID Serval
serval:BIB_572628EF6E09
DOI
10.1093/jat/28.6.426
PMID
15516291
WOS
000223630500008
Permalien
https://iris.unil.ch/handle/iris/74180
Open Access
Oui
Date de création
2008-02-08T16:44:47.325Z
Date de création dans IRIS
2025-05-20T16:32:30Z
Fichier(s)
En cours de chargement...
Vignette d'image
Nom

REF.pdf

Version du manuscrit

published

Taille

562.88 KB

Format

Adobe PDF

PID Serval

serval:BIB_572628EF6E09.P001

URN

urn:nbn:ch:serval-BIB_572628EF6E098

Somme de contrôle

(MD5):73a968074fcc5330ea97ee6e105a84b7

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